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Catechol-3-O-semiquinone (catechol-SQ) and 2-Hydroxychromone-3-O-semiquinone (2-OH-Chrom-SQ) were prepared by the photo-induced oxidation of catechol and 2-hydroxychromone, respectively, with the aim of determining the chemical behaviour of these molecules during the trimethylation of catechol-SQ and 2-OH-Chrom-SQ. The presence of pentaethylene glycol (PEG) as a solvent of catechol-SQ and 2-OH-Chrom-SQ leads to non-radical reactions and the formation of alpha-(hydroxymethyl)-tetrahydro-beta-carbolines (alpha-HMT-BCs). In addition, it was observed that 2-OH-Chrom-SQ is a more reactive species than catechol-SQ. The present results show that during the trimethylation, 2-OH-Chrom-SQ is converted to the alpha-HMT-BC precursor, whereas catechol-SQ is converted to an alpha-methylated tetrathiafulvalene (alpha-MeTTF-1) derivative. The kinetic analysis of the reactions of catechol-SQ and 2-OH-Chrom-SQ with pentaethylene glycol was achieved using the high performance liquid chromatography with ultraviolet (UV) detection (HPLC-UV) and fluorescence (HPLC-FL) techniques. The formation of alpha-HMT-BC and alpha-MeTTF-1 was confirmed by liquid chromatography coupled with electrospray ionization and atmospheric pressure chemical ionization mass spectrometry (LC/APCI-MS) techniques.We can today confirm the results of our Fan’s Choice in both
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